The monkeyspeak amulet mould is used in the Monkey Madness quest to make a monkeyspeak amulet. Zooknock requires this item, monkey dentures, and a gold bar to create an enchanted bar. The bar is then brought to the dungeon below the temple and is used on a magical flame along with the monkeyspeak amulet mould to create an monkeyspeak amulet which you then string with a ball of wool.
In order to get the mould you need to go to the building east of the magic stall on Ape Atoll. If you don't already have a greegree, you must stay in the dark area. Search the southeastern most crate to uncover a hidden entrance into the Temple of Marimbo Dungeon. Dropping down this entrance may yield some significant damage. Watch out for spiders, as they can poison. In the northwest corner there's a cluster of crates around a stalagmite; the moulds are in the crate directly south of the stalagmite.
After Monkey Madness, the monkeyspeak amulet mould can be bought at Hamab's Crafting Emporium for 10 coins.
The mould is later used in the Do No Evil quest to make a choc-ice in the shape of a monkey, called chimp ice.
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